From 4e73e452d1480c837de9fe063c1d8af1629ca3f6 Mon Sep 17 00:00:00 2001 From: ciuccislab Date: Sun, 5 Jan 2020 17:15:09 +0800 Subject: [PATCH] update --- README.md | 2 +- 1 file changed, 1 insertion(+), 1 deletion(-) diff --git a/README.md b/README.md index 05abb21..fcf51f0 100644 --- a/README.md +++ b/README.md @@ -1,7 +1,7 @@ # Project GP-DRT: Gaussian Process Distribution of Relaxation Times -This repository contains some of the source code for the paper "The Gaussian Process Distribution of Relaxation Times: A Machine Learning Tool for the Analysis and Prediction of Electrochemical Impedance Spectroscopy Data" https://doi.org/10.1016/j.electacta.2019.135316, which is also available in the [docs](docs) folder. +This repository contains part of the source code for the paper "The Gaussian Process Distribution of Relaxation Times: A Machine Learning Tool for the Analysis and Prediction of Electrochemical Impedance Spectroscopy Data" https://doi.org/10.1016/j.electacta.2019.135316, which is also available in the [docs](docs) folder. # Introduction Distribution of relaxation times (DRT) [1] method offers an elegant solution to analyze the electrochemical impedance spectroscopy (EIS) data encountered in material science, electrochemistry, and other related fields. However, deconvolving the DRT from the EIS data is an ill-posed problem [2-3], which is particularly sensitive to experimental errors. Several well-known approaches [2-5] can overcome this issue but they all require the use of ad hoc hyperparameters. Furthermore, most methods are not probabilistic and therefore do not provide any uncertainty on the estimated DRT. GP-DRT [6] is our newly developed approach that is able to obtain both the DRT mean and covariance from the EIS data, it can also predict the DRT and the imaginary part of the impedance at frequencies not previously measured. The most important point is that the parameters that define the GP-DRT model can be selected rationally by maximizing the experimental evidence. The GP-DRT approach is tested with both synthetic experiments and “real” experiments, where the GP-DRT model can manage considerable noise, overlapping timescales, truncated data, and inductive features.