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FFR_chap10.txt
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CHAPTER 10
HOMOGENEOUS REACTOR COST STUDIES*
10-1. INTRODUCTION
10-1.1 Relation between cost studies and reactor design factors. The
power cost associated with a reactor station may be subdivided into fixed
charges, operating and maintenance costs, and fuel costs. Fixed charges
include interest on investment, depreciation, and taxes; labor, supervision,
and maintenance are included in the operating and maintenance costs;
fuel costs include both variable and fixed chemical processing costs,t cost
of feed materials, and inventory charges. Because of the uncertainty of
these items, it is impossible to determine absolute costs for nuclear power
until large nuclear plants have been built and operated. However, it is
important that a reasonable effort be made to evaluate the cost in order to
compare several fuel or reactor systems of equal technological development,
to point out areas where substantial improvements are required, and to
provide a basis for determining whether economical power can ever be
produced.
Aqueous homogeneous reactors have certain features, such as high neu-
tron economy and continuous fission-product removal, which make them
appear to be potential economic power producers. However, as with all
water-moderated reactors, to attain steam temperatures corresponding to
thermal efficiencies of 25 to 30%, circulating aqueous systems require
operating pressures between 1000 and 2000 psia. Since thermal efficiency
increases relatively slowly with increasing operating pressure, while reactor
costs rise relatively sharply above pressures of about 1500 psi, it is unlikely
that reactors will be operated at pressures above 2000 psia. In addition,
icreasing the reactor temperature tends to decrease the breeding ratio,
which adversely affects fuel costs. Nearly all reactor systems considered
have therefore heen assumed to operate at pressures between 1500 and
2000 psia.
In order to optimize the design of a homogeneous reactor of a given
power output and pressure, it is necessary to know how both the fixed and
operating costs vary with the dimensions of the reactor core and pressure
vessel. In this regard, one must take into consideration that the maximum
diameter of the pressure vessel will be limited by fabrication problems, and
the minimum diameter of the core vessel will be limited by corrosion
*By P. R. Kasten, Oak Ridge National Laboratory.
TThe fixed costs in a chemical processing plant are those due to plant investment;
variable costs are due to materials, labor, ete.
514
10-1] INTRODUCTION 515
problems. For each combination of core- and pressure-vessel diameters
within these limits, there will be a mmimum fuel cost resulting from a
balance of inventory costs, processing costs, and tuel-feed costs; these latter
costs are determined by the breeding ratio, which is a function of fuel con-
centration and processing rate.
Although the fuel-fluid temperature influences power costs, this is nor-
mally limited by the properties of the fuel system or by the above-mentioned
pressure limitations, rather than by economic considerations. However,
the temperature range established on this basis is also close to that which
gives minimum fuel costs. In addition, the power level of the reactor is
usually assumed to be constant, although it is realized that this is a very
important factor influencing the cost of power, since plant investment
charges per unit power constitute a large fraction of the power cost and
change appreciably with power level. The effect of power level on capital
costs 1s discussed in Section 10-8, and on fuel costs in sections as noted.
The operating and maintenance costs, as well as plant investment costs,
are a funetion of reactor type and method of maintenance. However, the
exact form of some of the interrelations between design variables is not
known at the present time. For example, the plant investment and main-
tenance costs are undoubtedly different for a burner-type reactor than for
a breeder-type reactor; a cost difference would also exist between one- and
two-region systems. However, because of the lack of information, most
economic studies do not consider such differences, but assume investment
and maintenance charges to be determined primarily by the reactor power
level. The results of such studies are still significant if they are considered
in the light of the assumptions used; as more cost data are accumulated,
the results can be modified as required.
With respect to the fuel eycle costs, established Atomic Energy Commis-
sion prices for thorium, natural uranium, U232 and Pu®*, and the schedule
of charges for urantum of varying enrichments [1] provide a basis for cost
calculations. Charges for various chemical conversion steps and for proe-
essing spent fuel in a multipurpose chemical plant have also been an-
nounced [2]. Although these charges are applicable to the processing of
aqueous fuels, the possibility of including on-site processing facilities as part
of the homogeneous reactor complex must also be considered, since this
would have an effect on the reactor design.
10-1.2 Parametric cost studies at ORNL. The homogeneous reactor
systems considered include one- and two-region reactors, breeders, con-
verters, and burners. Although no one fuel or type of reactor shows a
marked advantage in power cost over all the others, the superior fuel
utilization of a thorium breeder system suggests that it is potentially the
most economical one for power production. Much effort has been devoted
516 HOMOGENEOUS REACTOR COST STUDIES [cHAP. 10
to two-region systems primarily because of the relatively high breeding
ratio and low fuel inventory obtainable.
Economic evaluations discussed in this chapter are for the most part
based on a three-reactor station generating a total of 375 Mw of elec-
tricity, where the required chemical processing facilities are shared by the
three reactors. The present choice of reactor dimensions for a given power
capability must be based on engineering judgment and the results of fuel-
cost studies. Based on fuel-cost studies, one-region reactors must be large
(14- to 15-ft diameter) in order to obtain good neutron economy; two-
region systems can have good neutron economy in relatively small sizes
(9- to 10-ft over-all diameter) but require high concentrations (1000 g/liter)
of fertile material in the blanket region. Iistimates of near-optimum reactor
sizes for different homogeneous systems are based on fuel-cost studies in
which highly enriched fissionable fuel 1s valued at $16/g and inventory
charges are 4%,. In all cases it is assumed that the particular fuel system is
technologically feasible.
In computing the cost of power, the fixed charges on capital investment
of depreciating items are assumed to be 159 /yr, including depreciation,
interest, return on investment, insurance, and taxes. Iixed charges on
nondepreciating items are assumed to be 49, /yr. Tuel, D20, and fertile
materials are assumed to be nondepreciating materials.
10-2. Bases ForR Cost CALCULATIONS
10-2.1 Fuel costs. The fuel costs associated with electrical power pro-
duced from reactors include those charges which are due to replacement of
conventional fuels with nuclear fuel. The fuel cost is considered to be the
sum of the net cost of nuclear-fuel feed; inventory charges for fertile mate-
rial, heavy water, and fuel; material losses; variable fuel-processing
charges; and fixed charges for fuel processing. Fuel-cost studies are pri-
marily for the purpose of investigating the economic importance of the
several parameters; of these parameters the most important are core
diameter, blanket thickness, fertile-material concentrations in core and
blanket, fuel concentration in the blanket, and poison fraction in the core.
In studying fuel costs, aqueous homogeneous power reactors are generally
considered to operate at a temperature of 280°C, a pressure 1500 to 2000
psia, an 809, load factor, and a net thermal-to-electrical efficiency of about
259,. The thermal power level per reactor i1s considered to be 450 to 500
Mw. Thorium (as oxide) i1s valued at $5/Ib with no significant charge for
making ThO2-D.0 slurry. Heavy water is valued at $28/Ib and highly
enriched figsionable uranium at $16/g. The amount of heavy water re-
quired 1s estimated on the basis of the total reactor-system volume and the
room-temperature density of heavy water. The makeup rate is taken as
10-2] BASES FOR COST CALCULATIONS 517
5%, vr. The volume of the core circulating system is taken as the volume
of the core plus an external volume of 1 liter for each 20 kw generated n
the core. The blanket external volume (in two-region reactors) is caleu-
lated on the basis of 1 liter for each 14 kw generated in the blanket. The
cost. of natural uranium 1s taken as $40/kg U either as UQy3 or U030y,
The cost of uranium of various enrichments in U39 13 obtained essentially
from the ALC price schedule or the equations for an ideal gaseous-diffusion
plant {3-5].
Fuel costs are dependent upon the value assigned to plutonium and U233,
In a power-only economy the value of these fissionable materials can be
no more or less than their fuel value; in these studies their value was taken
to be the same as that for U35 or $16/g. However, it U3 and/or plu-
tonium are assigned different values, the fuel costs can be significantly
affected. Thiz is shown m the results given for plutonium producers, in
which a plutonium value of $40/g was assumed (this value is consistent
with the ability of homogeneous reactors to produce plutonium containing
less than 29, Pu®*, and the AEC guaranteed fair price schedule for plu-
tonium extending until June 30, 1963).
The fuel values used in these studies are slightly different from those
announced by the AEC; the main difference is associated with the value
used for plutonium. However, the effect of various plutonium values on
fuel cost is indicated in the section on plutonium producers. The AEC-
announced prices for nuclear materials are given in Table 10-1.
Since the rate of fuel burnup is small with respect to the inventory of
fuel required for criticality, the investment and inventory charge for fuel
materials can be appreciable. Unless otherwise specified, inventory charges
for uranium, thorium, plutonium, and heavy water are assumed to be 4%,
of their value per year.
An economic consideration in the design of nuclear power plants is the
chemical processing requirement of the spent nuclear fuel. Aqueous
homogeneous reactor fuels can be processed by either the Purex or the
Thorex process. Both involve solvent extraction and require that the
fuels be separated from the D»0O for economical processing. The Purex
process is used for separating plutonium, uranium, and fission-product
poisons, while the Thorex process is used for the separation of thorium,
uranium, and fission products. Since investment costs in chemical process-
ing plants are presently high, a single processing plant for one good-sized
reactor is not economical. Rather, central processing facilities which serve
many reactors are usually assumed to be available. In the fuel-cost studies
given here, however, the chemical processing plant is considered to serve
a single three-reactor station generating about 1440 thermal Mw (total).
For this size processing plant, the fixed charges (based on 159, of invest-
ment per year) are estimated to be about $5500/day for either Purex or
518 HOMOGENEOUS REACTOR COST STUDIES [cHar. 10
TaBLE 10-1
U.S. AEC OrriciaL PrRICE SCcHEDULE FOR
NvUcLEAR MATERIALS [1]
(a) Price schedule of U235 as a function of enrichment
7 141 T235
W t(fdl;a%;?:) v $/kg total U $/gm U235 content
0.0072 40.50 5.62
0.010 75.75 &.09
0.020 220.00 11.00
0.030 375.50 12.52
0.10 1,529.00 15.29
0.20 3,223 00 16.31
0.90 15,361.00 17.07
(b) Price schedule of Pu as a function of Pu?#0 content
9 Pu20 ‘ Pu price, $/gm
2 1 41.50
4 38.00
6 34 .50
>8.6 30.00
(¢) Chemical conversion costs
Conversion Cost, $/kg
Uranyl nitrate = Ul
(U containing 59, or less by weight of T239) 5.60
Uranyl nitrate = UFg
(U containing greater than 59 by weight of U235) 32.00
Plutonium nitrate —- metal buttons 1,500.00
UFs (natural U) to oxide Zer0
(d) Valite of U233 (high purity) $15/g
10-2] BASES FOR COST CALCULATIONS 519
Thorex (complete decontamination) [6,11]. This corresponds to a power
cost due to chemical plant investment of 0.76 mill/kwh (based on a 375-Mw
net electrical capacity and an 809, load factor), which will be independent
of the amount of material processed daily.
The variable processing charges arising from labor, materials, and other
factors dependent on the throughput of fuel and fertile material are repre-
sented by Egs. (10-1) and (10-2) for processing thorium-uranium mixtures
and uranium-plutonium mixtures, respectively.
Thorex process
Variable daily processing cost = $3.00 Wy, 4+ 0.50 wy + 0.35 rp,o. (10-1)
Purex process
Variable daily processing cost = $3.50 Wy + $1.00 wp, + 0.35 vp,0. (10-2)
In the above equations:
vp,0 = liters D20 recovered/day,
wpy = ¢ Pu handled separately from U per day,
wy = g U processed per day,
W = kg Th processed per day,
Wy = kg U completely decontaminated per day.
Thus, for Thorex, the variable processing charge is considered to be
$3.00 'kg of thorium processed, plus $0.50/g total uranium processed
(U highly enriched in U233 4+ U23%), plus $0.35/liter of D20 recovered.
Note that Eqs. (10-1) and (10-2) take into consideration the effect of
throughput of fissionable material as well as fertile material on the variable
processing charges in a chemical plant of fixed size. This information Is
necessary in determining the optimum concentrations of fissionable and
fertile material in a reactor of specified dimensions.
The total processing cost in an on-site chemical plant, such as that
described above, will be 0.76 mills 'kwh plus the variable processing charges
and minus the credit for any net fissionable material produced. Thus the
chemical-plant investment costs exert a strong influence on the fuel costs.
These costs are lower if a large multipurpose chemical plant is available to
handle the fuel instead of the on-site plant. Fuel processing charges [2]
have been announced by the United States Atomic Energy Commission
for processing in such a multipurpose plant. These charges amount to
$15,300 per day, and apply to a plant having a daily capacity of 1 ton if
slightly enriched uranium (less than 3% U23% by weight) is processed, or a
daily capacity of 88 kg if highly enriched uranium is considered. In terms
of cost per gram of U2 processed, the above processing charges are
H20) HOMOGENEOUS REACTOR COST STUDIES [cHar. 10
equivalent to $2.15 per gram of U232 for natural uranium, $0.51 per gram
of U3 for uranium of 3% enrichment, and $0.37 per gram of U235 for
uranium of 479 enrichment. These values can be compared with those
considered previously, namely: $0.50 per gram of total uranium processed
(the enrichment of the uranium in the highly enriched systems is about
5090), and $3.50 per kilogram of natural or slightly enriched uranium
(equivalent to $0.50 per gram of U23% in natural uranium) plus $1.00 per
gram of plutonium. Thus, in most cases, the AEC total processing charges
amount to less than the variable processing charges considered here. In
case of a central processing plant, however, it would be necessary to in-
clude fuel-shipping charges and charges associated with preparing the
processing plant for the specific fuel.
In studying the poisoning effect of fission fragments, three groups of
fission-product poisons are considered. The first group consists of gases;
the second, nongaseous fission fragments having high microscopic cross
sections (greater than ~10,000 barns); and the third is composed of non-
gaseous fission fragments having low microscopic cross sections, and which
transmute to nuclides having the same low cross section. For processing
rates which do not cause excessive variable processing costs, only the third
group of poisons is affected by chemical processing; the first group is re-
moved by means other than Thorex or Purex, while the second group at-
tains equilibrium through neutron capture.
In processing U-Pu systems, a 20-day cooling period takes place hefore
processing 1 a Purex plant. Following complete decontamination, the
uranium is permitted to cool 100 more days before being re-enriched in a
diffusion plant. This 120-day holdup and also a 30-day feed supply are
considered in calculating inventory charges. In processing thoria slurries
(core region), the holdup time prior to processing i1s considered to be 95
days, to permit about 909 of the Pa233 to decay to U233, The processed
material is then held for an additional 110 days to permit the remaining
Pa233 to decay. For thoria slurries in blanket regions, an initial holdup of
55 days is assumed prior to processing, with an additional 150-day holdup
to permit the Pa23? to decay to U233, Thus the protactinium is held up for
205 days, in which time only about 0.5% has not yet decayed. This holdup
time and a 30-day feed supply are considered in caleulating material in-
ventories. Protactinium is valued as uranitum when outside the reactor,
but no inventory charge is placed against the amount contained in the
reactor system. This procedure is used to take into account that period of
reactor operation between startup and near-equilibrium conditions. Unless
otherwise indicated, the results are based on the assumption that equilib-
rium exists with respect to the nuclei concentrations. The isotope and
fuel concentrations are established by means of material-balance equations
and the critical equation.
10-3] FUEL COSTS IN THO2-UQ3 D20 SYSTEMS 521
In nearly all cases, fuel concentrations required for criticality are ob-
tained using the two-group model [7], in which all fissions are assumed to
oceur in the thermal group [see Eqs. (2-7) through (2-10)]. Resonance
capture is assumed to occur only in fertile material and only when neutrons
are transferred from the fast to the slow group. For the one-region U-Pu
systems, a six-group model is used in the nuclear calculations to allow for
the resonance absorptions in uranium and plutonium. Unless otherwise
specified, the thermal values for the various etas are n(U233) = 2.25,
n(U23%) = 2,08, n(Pu??) = 1.93, and n(Pu?*!) = 2.23.
10-2.2 Investment, operating, and maintenance costs. The costs con-
sidered here involve capital investment, and those associated with main-
taining and operating the nuclear power plant. Becau=e of the lack of
knowledge and experience in design, construction, and operation of nuclear
power systems, it is difficult to evaluate these costs, and most estimates
are based on the expectation that nuclear reactor plants will have lifetimes
about as long as those of conventional power plants. A 20-year depreciation
rate is assumed for permanent facilities and a 10-year depreciation rate for
all equipment associated with the reactor proper. Preparing a realistic
estimate of the cost and the required maintenance of a large homogeneous
reactor ig particularly difficult, since the equipment must handle large
amounts of radioactive material. Little experience has been obtained in
manufacturing the required equipment, and generally the costs are based
upon estimates by manufacturers. These estimated costs of equipment for
a specific reactor power are scaled according to the reactor power raised
to the 0.6 power to obtain the variation of investment cost with power
level. The annual operating and maintenance charges have been estimated
by roughly applying the corresponding charges (based on percentage of
:apital investment) in conventional steam plants; however, these estimates
cannot be considered realistic until considerable experience has been ob-
tained by operating actual reactors. These estimates correspond to 3%
of the total capital investment per year.
10=3. Errect oF DEsioN VARIABLES oN THE FueL Costs
N THO2-UO3-D20 SysteEMms [8-10]
10-3.1 Introduction. Fuel costs are given here for spherical two-region
reactors with UZ303—ThOs D»0O slurry employed in both the core and
blanket regions. Results are also given for the case of no thorium in the
core and also for one-region reactors. In addition, some results are given
for two-region reactors having cylindrical geometry. In the two-region
systems, materials from the core and blanket are assumed to be fed to a
Thorex plant for chemical processing. Thoria can be returned to both
522 HOMOGENEOUS REACTOR COST STUDIES [cuaP. 10
Feed D,O Makeup Thorium Feed
30 Days
Feed D20 Supply on Supply ofl
Storage Thorium
‘ Core -— Core Blanket —={ Blanket
Reactor u External External
System e
Volume g - Volume
Core *Poison Hydroclone Separation
Rem'ovcl of Fission Products
D50
Recovery I DZO Evaporation ——
Pre-Chemical o Core Blanket Holdup,
p i and Initial
r:cnla:smg ;'lo|dup, Additional Processing
oldup 5 Days Holdup, 55 Days
150 Days Pa
________________ U_ — - —-——
] Y
Core Blanket
Chemical Chemical
Chemical Processing ~__Processing
Processing u I Poisons Poisons U Th {
Products Fission Products Net Uranium
Production
High Purity y233
Fig. 10-1. Schematic fuel-processing flowsheet for a two-region homogeneous
thorium breeder reactor.
regions and fuel is returned to the core as needed to maintain criticality;
the fissionable material produced in excess of that required is considered
to be sold. The fuel product is computed to be a mixture of U233 235
and other uranium isotopes, as determined by the isotope equations and
the critical equation. The system is assumed to operate under equilibrium
conditions. A schematic flowsheet of the chemical processing cycles for a
two-region reactor having a solution-type core region is given in I'ig. 10-1.
The flowsheet for the one-region system would be similar to that for the
blanket of the two-region system, except that processed fuel and thoria
would be returned to the single region.
In the processing cycle shown in Fig. 10-1, essentially two methods of
removing fission-product poisons are considered. One is the removal of
precipitated solids by hydraulic cyclones (hydroclones); by this means
the insoluble fission products are removed from the reactor in a cycle time
of about a day. The second is the removal of essentially all fission produects
10-3] FUEL COSTS IN THO2-U03-D20 SYSTEMS 523
by processing tne fluid in a Thorex-processing plant. Processing by hydro-
clones can he done only with solution fuels; the associated cyele time 1s so
short that fission products removed by this method ean be considered to
he removed from the reactor as soon as they are formed. Thorex processing,
although removing all fission products that pass through Thorex, 18 much
more costly than hydroclone processing. Because of this, the associated
cyele time 18 usually several hundreds of days. In what follows, unless
specified otherwise, the term fuel processing applies only to Thorex or
Purex processing,
The essential difference between the processing eycele shown m Fig., 10-1
and that for solid-fuel reactors 1s assoctated with the continuous removal
of fission-product gases and of insoluble fission products (in solution re-
actors). I‘uel and fertile material processed by Thorex would undoubtedly
be removed from the reactor on a semibatch basis.
The three groups of fission-product poisons considered previously are
not all affected by Thorex processing; group-1 poisons (the fission-product
gases) are assumed to be physically removed before processing, while
group-2 poisons (nongaseous nuclei having high cross sections) are effec-
tively removed by neutron capture within the reactor system (¢, of these
nuclel 1s of the order of 10,000 barns). The macroscopic cross section of
these two groups of poisons is taken as 1.897 of the fission cross section.
Of this, 0.89, is due to nongaseous high-cross-section nuclel, while 144 is
due to the gaseous high-cross-section nuclei. The concentrations of low-
cross-section nuclei (third group) are affected hy Thorex processing (how-
ever, for reactors containing a fuel solution, the nonsoluble group-3 poisons
are assumed to be removed by hydroclone separation). The charge for
hydroclones operating on a olie-day cycle is taken as 0.03 mill,/'kwh, based
upon a charge of $75/day per reactor. Ior these solution reactors it 1s
assumed that 759, of the group-3 poisons are insoluble and removed by
hydroclones; in these circumstances only 259; of the generated group-3
poisons are removed by the Thorex process. With slurry-core reactors, all
group-3 poisons which are removed are removed by Thorex processing.
The parameter ranges covered in the spherical reactor calculations are
given in Table 10-2. Values used for n*? and resonance escape probability
are presently accepted values; however, in a few cases they were varied in
order to estimate how the results are affected by these changes. In the
following sections the influence of specific parameters upon fuel cost is
discussed.
10-3.2 Two-region spherical reactors [8]. (1) Concentration of U™3 in
blanket and core poison fraction. The optimum values of these variables are
found to be largely independent of other parameters; moreover, there is
little change in fuel cost with changes in either blanket U233 concentration
524 HOMOGENEOQUS REACTOR COST STUDIES [cmaP. 10
e ' | T
Net Fuel Cost
{mills/kw-hn
Blanket Thickness (f)
F1c. 10-2. Fuel cost as a function of blanket thickness for various blanket
thorium concentrations. Power per reactor = 480 Mw (heat), core diameter = 5 ft,
core thorium = 200 g/liter, core poison fraction = 0.08, blanket U233 = 4.0 g/kg
Th, 523 = 2.25,
or core poison fraction. For all slurry-core systems, the optimum poison
fraction is about 0.08, independent of the other design parameters. The
optimum poison fraction for the solution core is about 0.07. The lowest
fuel cost occurs at a blanket U233 concentration of about 4.0 g/kg thorium.
TaBLE 10-2
PArRaMETER VALUES UseED IN SLURRY REACTOR STUDIES
Two-region reactors | One-region reactors
Core diameter, ft 8-15 8-20
Blanket thickness, ft -3
Core thorium concentration,
g/liter 0-300 0-400
Core poison fraction, 9; 3-20 4-12
Blanket thorium concentration,
g/liter 500-2000
Blanket U233 concentration,
g/kg thorium 1-7
(2) Blanket thickness and blanket thortum conceniration. An example of
the effects of these parameters on fuel cost is presented in Fig. 10-2 for a
slurry-core reactor. Here it is noted that the blanket thorium concentra-
tion has relatively little effect on the minimum fuel costs. The blanket
thickness giving the lowest fuel cost lies between 2 and 2.5 ft. As is ex-
pected, higher thorium loadings are desirable if thin blankets are necessary
on the basis of other considerations. Systems having low concentrations of
thorium in the core require more heavily loaded blankets to minimize fuel
costs. For solution cores, still heavier and thicker blankets are desirable,
particularly if the core diameters are small.
10-3] FUEL COSTS IN THO2-UO3-D20 SYSTEMS 525
[ | |
Core Thorium|
{g/liter}
- —
-
-l
_____
Net Fuel Cost (mills /kw-hr)
i
3
4(2.5) 5{2) 612) 712}
Core Diameter (Blanket Thickness) (f8)
F1c. 10-3. Fuel cost as function of core diameter and core thorium concentration,
Power per reactor = 480 Mw (heat), blanket thorium = 1000 g/liter, blanket U233
= 4.0 g/kg Th, core poison fraction = 0.08, 23 = 2.25.
(3) Core thorium and core diameter. The effects of these variables upon
fuel costs are shown in Fig. 10-3. These results indicate (on the basis of
fuel cost alone) that the small solution-core reactors (ThOs core concen-
tration equal to zero) have a slight advantage over the slurry reactors.
However, the power density at the core wall is between 160 and 300 kw/liter
for such reactors operating at the given power level of 480 thermal Mw. If
larger cores are required because of power-density limitations, the fuel-cost
advantage moves to the slurry core. The slurry-core systems yield higher
outputs of generated fuel, although all the reactors shown have breeding
ratios greater than unity (see Chapter 2). As illustrated in Fig. 10-3, the
minimum fuel cost is about 1.2 mills/kwh, independent of core diameter.
The fuel cost associated with a core thorium concentration of zero is lower
than that associated with a core thorium concentration of 50 g/liter; this
is due to the ability to use hydroclones to remove fission products only
when a fuel solution is used. The hydroclone installation adds only
0.03 mill/kwh investment cost to the system, while the variable Thorex
processing cost is reduced by two-thirds; this results in the decrease in fuel
costs as shown. The relative flatness of the optimum net fuel cost curve in
Fig. 10-3 is due to compensating factors; i.e., changes in processing charges
and yield of product are offset by accompanying changes in the fuel in-
ventory charge. Similar compensating effects account for the insensitive-
ness of fuel costs to changes in other design parameters.
Table 10-3 presents a breakdown of costs for some typical reactors hav-
ing low fuel costs. The changes which occur when thorium-oxide slurry is
526 HOMOGENEOUS REACTOR (OST STUDIES [cHAP. 10
Tasri 10-3
Cost BrEAKDOWN FOR SoME Typican REACTORS
Core diameter, ft 6 5 4 6 14
Blanket thickness, ft 2 2 24 2 i
Core thoriuin concentration,
g/liter 200 100 0 0 250
Blanket thorium concentration,
g /liter 1000 1000 1000 1000
Blanket U232 concentration,
g/kg thorium 4 4 4 4
Core poison fraction 0.08 0.08 0.08 0.08 0.08
Critical concentration,
g U238 liter 9.4 |64 |41 14 |68
Net breeding ratio 1,102 | 1.081 | 1.089 | 1.045 | 1.012
Core wall power density, kw/liter | 53 91 170 80
Core cycle time, days 637 418 884 342 1094
Blanket cvcle time, days 265 205 176 210
Inventory of U2 and U235 kg | 368 272 200 148 522
Inventory of heavy water, Ib 96,100 | 87,400 @ 89,600 | 99,500 | 157,000
Net U2 and U235 production,
o/day 49 39 43 21 6
Grams of U233 per g of U pro- j
duced 0. 67 0.65 0.77 (.72 0.41
Estimated cost, mills/kwh
Uranium inventory 0.27 0.20 0.15 0.11 0.38
D20 inventory and losses (.27 0.25 (.25 0.29 0.45
Thorium inventory and feed 0.01 0.01 0.01 0.01 0.01
Fixed chemical processing 0.76 0.76 0.76 0.76 0.76
Core processing 0.13 0.13 0.07 0.08 0.19
Blanket processing 0.09 0.12 0.18 0.18
TUranium sale, credit 0.33 0.26 0.29 0.15 0.04
Net fuel cost 1.22 1.22 1.16 1.29 1.76
used in the core can be seen by comparing results for the two 6-ft-core-
diameter reactors.
(4) Reactor power. The above results are based on the concept of a three-
reactor station of 1440-thermal-Mw capacity, each reactor producing
125 Mw of electricity. The effect of varying power alone is shown in
Table 10-4; the fuel cost is found to be a strong function of power capa-
bility. The greater part of the change is due to variation in the fixed
chemical-processing charge. Since the total fixed processing cost
($5500/day) is assumed to be independent of throughput, this charge on
a mills/kwh basis is inversely proportional to the reactor power.
10-3] FUEL COSTS IN THOo—UO3—D20 SYSTEMS 527
TavLr 104
Errect oF Power LeveL ox I'uen Costs
Ileetric power per Net fuel cost, lj]"fe(‘i .('hen;u':?l.-
reactor, Mw mills ‘kwh pl()(,es'smg Charse,
’ mills/kwh
80 1.75 1.19
125 1.22 0.76
200 0.88 0.48
(5) Nuclear parameters. The values of n(U?%) and the resonance escape
probability of thorium-oxide slurries are not known with certainty. There-
fore the etfects of changes in these parameters on the results were com-
puted in order to examine the reliability of the nuclear caleulations. The
fuel cost increases by about 0.2 mill/kwh if %% is changed from 2.25 to
2.18, and 1s reduced by about the same amount if the 23 value is taken to
be 2.32 rather than 2.25.
The importance of resonance escape probability for thoria-D»O slurries
(p") upon fuel cost was studied by using values for (1 — p®) which are
209, higher or lower than a standard value. With a core thorium concen-
tration of about 200 g/liter, the changes in p®? have a negligible effect upon
fuel cost. At lower core thorium concentrations, the changes in p°2 result
in fuel-cost changes of about (.05 mill /kwh.
(6} Xenon removal. For most of the cases studied, the contribution of
xenon to the poison fraction is assumed to be 0.01. To achieve this condi-
tion, about 80% of the xenon must be removed before neutron capture
occurs. Since xenon-removal systems for slurries have not been demon-
strated to date, the effect of operating without xenon removal was studied
by increasing the xenon poison fraction to 0.05 (the samarium contribution
was held at 0.008). In the systems examined, when the xenon poison frae-
tion was increased by 0.04, the total poison fraction yielding the lowest fuel
cost also increased by approximately the same amount. The values in
Table 10-5 illustrate this etfect by comparing two cases at optimum total
poison fraction, but at different xenon poison levels. Thus the variable
part of the core poison fraction (and the core processing rate) remains about
the same. The higher fuel cost at the higher xenon level appears to be al-
most entirely a result of the reduction in breeding ratio.
10-3.3 One-region spherical reactors [8]. (1) Poison fraction. The
poison fraction producing the minimum fuel cost for a given system is in
the range from 0.06 to 0.10, the exact value depending on the specific di-
528 HOMOGENEOUS REACTOR COST STUDIES [cHAP. 10
2.4
\ |
Core Diameter (ft) 18
2.2 1—
&=
3
-
%
E 20| 1
E 10
o
2 14
% 18— 1
z
1.6 | | | l | \
50 100 150 200 250 300 350 400
Thorium Concentration, g/|i1er
Fra. 10-4. Fuel cost as function of thorium concentration in one-region reac-
tors. Power per reactor = 480 Mw (heat), poison fraction = 0.08, %3 = 2.25.
ameter and thorium concentration. However, a value of 0.08 gives costs
which are close to the minimum for all cases.
(2) Diameter and thorium concentration. The fuel costs for some of the
single-region reactors studied are shown in Fig. 10-4. Detailed information
TaBLE 10-5
ErrFect oF XENON PoisoN FractioNn oN FuerL Costs
Xenon poison fraction 0.01 0.05
Optimum total poison fraction 0.08 0.12
Core cycle time, days 637 718
Breeding ratio 1.102 1.070
Fuel inventory charge, mill/kwh 0.27 0.29
Core processing charge, mill/kwh 0.13 0.14
Fuel product (credit), mill/kwh 0.33 0.22
Net fuel cost, mills/kwh 1.22 1.35
for a typical one-region reactor is given in the last column in Table 10-3.
In general, for thorium concentrations less than 400 g/liter the reactor
diameter must be greater than 10 ft in order to have a breeding ratio greater
than unity; the 12-ft-diameter reactor is a breeder (breeding ratio = 1.0)
at a thorium concentration of 350 g/liter, while at 250 g Th/liter the
14-ft-diameter reactor is a breeder. For reactors between 10 and 16 ft in
diameter, the thorium concentration yielding the lowest fuel costs is be-
10-3] FUEL COSTS IN THO2-UO03-D20 SYSTEMS 529
tween 200 and 275 g/liter. The lowest fuel cost is about 1.76 mills/kwh
(for a 14-ft-diameter reactor containing 270 g Th/liter). In the curve for
the 14-ft reactor, the inflection in the neighborhood of 225 ¢ Th/liter is a
result of the reactor changing from a breeder to a nonbreeder. This in-
flection is associated with a marked increase in U236 concentration (concen-
trations are based on equilibrium conditions), which produces an increase
in fuel processing charges (in all cases it is assumed that U233 is fed to
the system).
(3) Power and nuclear parameters. The effect of reactor power on the
fuel costs of one-region reactors is similar to that mentioned earlier for
two-region systems. For example, if the total fuel cost for a three-reactor
station is 1.76 mills/kwh at 125 Mw of electric capability per reactor, it
would be only 1.38 mills/kwh if the output per reactor were increased to
200 Mw,
The importance of changes in nuclear parameter is generally the same
for the one-region reactors as for the two-region systems, although the
effect upon fuel costs of a reduction in n(U?33) is somewhat greater for the
one-region cases.
10-3.4 Cylindrical reactors [9]. The effects of geometry on fuel cost
are due to the associated changes in inventory requirements and breeding
ratio. Accompanying these effects are changes in the average power den-
sities and the wall power densities within the reactor. Because of corrosion
difficulties associated with high power densities, it is desirable to operate
with reasonahly large reactor volumes. Cylindrical geometry permits re-
actors to have large volumes without necessitating large reactor diameters.
One-region spherical reactors would have to be large in order to prevent
excessive neutron leakage, and so power densities would not be high
(average power densities of about 30 kw/liter). Also, closure problems
with respect to maintenance of an inside vessel would not exist. Therefore
there is little incentive to increase reactor volume by using cylindrical
geometry for one-region homogeneous reactors.
For two-region reactors, cylindrical geometry may prove advantageous
with respect to feasibility and relative ease of reactor maintenance. How-
ever, the associated larger fuel inventories (in comparison to inventories
for spherical geometry) will increase fuel costs. Comparison of results for
two-region cylindrical reactors with those for spherical two-region reactors
shows that cylindrical geometry gives minimum fuel costs about
0.2 mili/kwh greater than does spherical geometry, if in either case there
were no restrictions on core-wall power density. The difference is even
greater if the core-wall power density influences the reactor size. However,
cylindrical geometry does permit low wall power densities in combination
with relatively small reactor diameters.
530 HOMOGENEOUS REACTOR COST STUDIES [cHAP. 10
]
Conversion of | Enriched U
Feed Preparation UF g to UO5
30-Day Reserve
U, Pu Feed