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FFR_chap24.txt
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FFR_chap24.txt
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CHAPTER 24
LIQUID METAL FUEL REACTOR DESIGN STUDY*
24-1. CompARISON oF Two-FLuip AND SINGLE-FLUID
LMFR DeEsignNs
In Chapter 18, the two-fluid and the single-fluid externally cooled LMFR
concepts were discussed in a general way. It was pointed out that the two-
fluid design has the better breeding possibilities but is somewhat more
complex than the single-fluid reactor. In this chapter a complete design
study of a two-fluid full-sized LMTR reactor is deseribed and discussed,
and a shorter discussion of a single-fluid design study follows. This does
not mean that one design is necessarily favored over the other. In fact
both of these designs are being studied very extensively.
24-2. Two-Fruip Rracror DESIGN
24-2.1 General description. The two-fluid externally cooled LMFR
concept consists of a relatively small core surrounded, for the most part, by
a blanket containing fertile material. The core is composed of high-density,
impervious graphite through which vertical channels are drilled to allow
circulation of the fuel coolant. The fuel in the core is dissolved U233 or
U233 dissolved and suspended in liquid bismuth. The fluid fuel also acts as
coolant for the core system. The required coolant to moderator ratio is
obtained by proper size and spacing of the fuel coolant channels.
The blanket is constructed of high-density graphite through which flows
a liquid bismuth slurry containing the bred U?2*3 fuel and thorium, the
fertile material. In this study, thorium is assumed to be suspended in bis-
muth as thortum bismuthide, although thorium oxide particles could be
used. The blanket is wrapped around the core as completely as possible
for good neutron economy. An important economic consideration is the
degree of end blanketing which can be achieved while keeping coolant
velocities below the allowable limit. Several blanket designs were in-
vestigated, but a complete study for obtaining the best end blanket design
has not yet been carried out.
*This chapter is based on studies made by Babeock & Wilcox Company for the
USAEC, BAW-1046, March 1958, and on a 17 company report BAW--2, June 30,
1955, for which Brookhaven National Laboratory contributed information and sup-
plementary design studies.
866
24-2] TWO-FLUID REACTOR DESIGN 867
24-2.2 General specifications. Unless otherwise noted, the specifications
listed below are common to all calculations performed in this design.
Total power 825 mw (thermal)
315,000 kw (electrical)
Coolant to moderator ratio in core, Vpi/Vc 1.22
Coolaut to moderator ratio in blanket, Vaury/Ve — 0.50
Core-blanket barrier material graphite
Blanket thickness 3.0 ft
Blanket slurry composition:
Bismuth 90 w/o
Thorium, as ThzBis 10 w/o
C'oolant inlet temperature 750°F
Coolant outlet temperature 1050°F
Nuclear ealeulations utilizing latest cross sections and multigroup diffu-
sion theory indicate that the values 1.22 and 0.50 listed above are close
to the optimum.
The =everal factors which dictated the choice of a bismuth-to-carbon
volume ratio merit some attention. There are some losses of neutrons due
to capture in graphite. Hence, one would wish to use only enough graphite
to <utliciently thermalize the reactor. If too little graphite is used, the
eritien] mass will be large. It is suspected that the % value for U23? may
be lower in the epithermal than in the thermal energy range. This would
nuke it desirable to keep the reactor thermal. It was found that bismuth-
to-carbon volume ratios in the range of 0.5 to 2.0 satisfy these various re-
quirements quite well. It may be further observed by referring to Iig. 24-1
thut breeding improves with an increase in the bismuth-to-carbon volume
ratio. However, the maximum bismuth-to-carbon volume ratio acceptable
on the basis of structural limitations was 1.22) and consequently this core
ditneter 15 155.7 em (61 in.) at a bismuth-to-carbon volume ratio of 1.22;
assiutning a cvlinder with its height equal to diameter.
Bianlt slurry-to-graphite volume ratio and blanket thickness. A series of
crliulitions were made to estimate the most economical parameter values
for the blanket. Blanket slurry-to-graphite volume ratio and blanket
thicknes=s were varied to give the best breeding ratio consistent with reason-
able hismuth holdup. Figures 24-2 and 24-3 demonstrate the effects of
varving blanket composition and thickness on breeding ratio. The slurry-
to-graphite volume ratio was set at 0.5 and the blanket thickness was set
at o1t
Studiy of design parameters. The parameters investigated in the following
analvsi= are (11 end blanket design, (2) power fraction in the blanket, and
(31 tizsion product poison level in the core.
868
0.14
0.12
0.10
o
o
®
Breeding Guain
o
o
>
0.04
0.02
LIQUID METAL FUEL REACTOR DESIGN STUDY [cHAP. 24
[ I | T I I
Noa/Ng. ~ 15 x 10 4
23" 7B
] ] ] | ] ] 1 1
0.25 0.50 075 1.00 1.25 1.50 175 2.00 2.25
Bismuth te Carbon Volume Ratio
F1a. 24-1. Breeding gain vs. bismuth-to-carbon volume ratio in core.
Breeding Ratio
1.1
0.9 l ] L
2.0 2.5 3.0 3.5 4,0
Blanket Thickness in Ft.
Fia. 24-2. Breeding vs. blanket thickness for slurry-to-carbon volume ratio
= 1.00 and bismuth to carbon volume ratio in core = 1.00.
Breeding Ratio
i i ! [ i
1.04
0.50 0.75 1.00 1.25 1.5¢ 175
Slurry to Carbon Volume Ratio
Fia. 24.3. Breeding vs. slurry-to-carbon volume ratio in blanket for bismuth to
carbon volume ratio = 1.00 and blanket thickness = 3 ft.
24-2] TWO-FLUID REACTOR DESIGN 869
24-2.3 End blanket effects. A series of nuclear calculations were per-
formed to determine the effects of end blanket design upon breeding ratio
and eritical fuel concentration. Two extreme blanket designs were con-
s1dered. In the most optimistie case, a spherieal core, equivalent to a 61-in.-
diameter eylinder, was surrounded by a 3-ft spherical blanket. The pessi-
mixtic caleulations assumed a cylindrical core with a diameter of 61 in.,
height equal to 1.5 times the diameter, a 3-ft radial blanket, and no end
blanket. Critical values of fuel concentrations and breeding ratio were
caleulated for four power fractions in the blanket for cach design.
All caleulations were performed for hot, clean conditions with an average
temperature of 900°I. A two-group, multiregion code was used to solve
the diffusion equations, and a 37-group spectral code was used to determine
the two-group nuclear constants. The results of these calculations are
taubulated in Table 24-1. The breeding ratio is decreased 0.20 to 0.25 by
completely eliminating the end blankets. This is due primarily to the
added neutron leakage out the ends of the core, despite the fact that the
core height 1s Inereased. Although the eritical mass of fuel in the core is
higher without end blankets, the fuel concentration is somewhat lower
due to the increased core volume.
TasLe 24-1
CriTicaniTy Cancurations rorR Two-I'wuip LMEFR
WITH AND WITHOUT IKND BLANKETS
Vay/Npi X 10° Ratio of . Blanket
‘ \ Breeding : .
(use ———— | blanket power ratio thickness, (ieometry
-~ Core | Blanket | to total power ' ft
I - 509 152 0.0665 1.053 3.0 Full blanket
IT 530 034 0.205 1.051 3.0 ? ”
1 461 | 1600 0.445 1.039 3.0 7 ”
IV 7 436 2100 0.515 1.033 3.0 7 "
V 403 1050 0.272 0.80 3.0 No end blanket
VI 366 2100 0.425 0.82 3.0 v ”
VII 347 2808 0.492 0.83 3.0 v !
VIIT' 403 | 1050 0.272 — 4.0 v "
The actual core and blanket design is between the two extremes assumed
in these caleulations. The blanket can be extended beyond the end bound-
aries of the core, and a graphite reflector can cover the ends of the core
except for the coolant inlet and outlet. Cooling becomes a serious design
870 LIQUID METAL FUEL REACTOR DESIGN STUDY [cHAP. 24
0
C ] | L shielding
'
Control Rod/ET ]
Control Rod Drive
]
/L
Core Qutlet
Nozzle ///// /// Blanket C])uflef
T
7
S
R A B R
R R SRR R
R R R R RS
NN
pSSSSE
TR
R R R R R R AR
TN
.
A R T
]
|
Fuef Passage Blanket Inlet
Nozzle
Core Inlet
Nozzle
FiG. 24-4. Two-region, externally cooled liquid metal fuel reactor.
problem, if the end reflector is replaced with blanket material. The design
in Fig. 24-4 is a substantial improvement over no end blanket or reflector.
However, further improvement in breeding ratio could be achieved with
even better end blanket designs.
24-2.4 Power level in the blanket. For a given geometry, coolant-to-
moderator ratio, and thorium concentration in the blanket, specification of
the fraction of total fissions generated in the blanket establishes a unique
set of values for fuel concentration in the blanket, fuel concentration in the
core, and fissions generated in the core. For simplicity, the power generated
in a region is assumed directly proportienal to the fissions in that region.
The data in Table 24-1 indicate that breeding ratio changes very little
with large changes in the fraction of total power generated in the blanket.
This increase in blanket power results in an Increased ratio of resonance
to thermal absorptions, a phenomenum which tends to offset the additional
fast neutron leakage out of the blanket as blanket power increases.
24-21 TWO-FLUID REACTOR DESIGN 871
An economic analysis of the effects of changing the blanket power frac-
tion was performed to determine the optimum core-blanket power split
under equilibrium operating conditions. The parameters affecting this
choice are (1) fission-product poison levels in the blanket, (2) fission-
product poison levels in the core, and (3) chemical processing costs,
Frission-product poisons in the blanket. The chemical processing of the
blanket slurry accomplishes two things:
(1) The removal of bred U?3? from the blanket system at a rate necessary
to maintain the 17232 concentration in the blanket slurry at some equilibrium
value corresponding to the desired blanket power fraction.
(2) The removal of fission products from the blanket slurry.
If the blanket processing cycle 1s determined by the minimum removal
rate of 17238 for steady-state operation, a corresponding poison level in
the blanket 1= automatically set. If the blanket chemical processing cyele
1= determined by the poison level and is less than the cycle determined by
the above criteria, the bred fuel removed from the blanket must be fed
hack into both core and blanket to maintain steady-state fuel concentra-
tions. In this analysis the blanket processing eyele i all eases was assumed
to be based on the minimum removal rate to maintain steady-state U233
concentrations without feeding fuel into the blanket system.
(e mical processing cycle for blanket slwrry. The chemical processing was
a==umed to be performed continuously on the reactor site. Unless other-
wise specified, the fluoride volatility process is utilized as described in
Article 24-3.16. The chemical processing cycle for the blanket may be
caleulated 3] from the equation
_ ZW Mg [V 4 (Z1a/ Z.) (0 a)]
s s — (07
T'p = blanket processing cycle, days,
Tg
where
Z, = removal efhciency for uranium = 0.25,
Z13 == removal efficiency for protactinium = 0.04,
M, = mass of fuel in blanket system, kg,
h, a = ratio of Pa®33 to U233 in blanket,
3 = kg of fuel burned per Mwd = 1.05(1 4+ «23),
P, = total power, 825 Mw,
BR = breeding ratio,
Pg = blanket power, Mw,
872 LIQUID METAL FULL REACTOR DESIGN STUDY [cHAP. 24
and
Z
Tg
¥
0% (efh)d™ +
Y13
Qe
where
0% (eff) = an effective absorption cross section to account for resonance
and thermal absorption in 17233
3
o5 = average thermal flux over the blanket system,
Y13 = decay constant for Pa®33,
The poison level in the blanket depends upon T, and Tg 1= a function
of M J, b/a, breeding ratio, and power fraction in the blanket. All these
arviables are interrelated. The ratio b,/a 1s a function of Ty, but Tpis a
slowly varying function of b/a due to the low value of Z,3/Z, (0.16).
Breeding ratio is a slowly varying function of fission-product levels in the
blanket due to the heavy loading of fuel and thorium in that regiow.
The breeding ratio is sensitive to the poison level, and thus to the chemical
processing rate, in the core fuel solution. An iterative calculation procedure
was required to arrive at optimum values of T, fission-product poison
level in the blanket, and the power fraction in the blanket.
For a given chemical processing rate in the blanket, the fission-product
poison level was determined from the data in KAPL 1226 [4]. Relative
poisoning, RP, is defined as the absorptions in fission products per thermal
fission in fuel, while the fission-product poison fraction is the absorptions
in fission products per total absorption in fuel. Xenon and samarium are
treated separately and are not included in the term fission products. The
burnup, F, in a region is defined as the atoms of fuel fissioned per atom
present in the region. The burnup F at time T in the blanket is caleulated
from
. 0.866 T(Pg/1IP)
F= - ;B
Mas
Using this relation, the relative polsoning in the blanket was determined
for ench processing cycle from a graph of R versus I7 [4]. The RP curve
used is based upon high cross sections of all fission products with the excep-
tion of u low value for Zr¥s,
Xenon in the blanket. Xenon is removed from the blanket by the degasser.
Although the removal rate of fission-product gases cannot be determined
until experimental information becomes available, a poison fraction of 0.01
was assumed for Xe!33,
24-2] TWO-FLUID REACTOR DESIGN 873
Samartum n the blanket, The removal rate of samarium by chemical
processing wus neglected. The steady-state ratio of Z50/Z3 using ap-
propriate thermal absorption cross sections, is determined by the relation
8
5
Som= 1.42 X 10716¢ + 0.0126,
where ¢ = average thermal flux in the region of interest.
Fisston-product poisons in the core. The level of fission products, FP,
other than xenon and samarium, in the core 1s determined by the chemical
processing cyele for the core fuel solution. The steady-state value of FP
poisons in the core should be established by an economie balance between
the value of improved breeding ratio and inereased chemical processing
costs, The relationship between the core processing cycle, T, and the rela-
tive poizon, RP, in the core may be expressed as
d(RP) _RP
dF ~ F
and
0.866 T.(P./P)
F=——
My,
where
D
d(;;‘}') 1s the slope of the curve RP versus F [4],
Mgy = total mass of U23? in the core system.
The xenon and samarium poisons in the core are determined as described
for the blanket.
[eonomie optimization. An optimization study was performed to de-
ternune the most economic power split between core and blanket systems
qind fission-product poison level for the core during equilibrium operation.
The tuel cost items which vary with these two parameters are (1) bismuth
Heventory. (29 fuel inventory, (3) fuel burnup, (4) thorium amortization,
5 thortum burnup, and (6) chemical processing. Nuclear calculations
specitied the fuel concentrations for both core and blanket and breeding
ritin=. These values were then used to determine the chemical processing
cvele for the blanket and the pertinent costs.
874 LIQUID METAL FUEL REACTOR DESIGN STUDY [cHAP, 24
2800
2600 -
2400 —
2200 |
2000 -
1800
1600 |—
Ngq/Np; in Blanket x 10®
5 ~ =
g8 8 8
|
o
o
<O
I
600 |~
400 -
200 —
Pg/Py
F1g. 24-5. Fuel concentration in blanket vs. Pg/P; for two-fluid LMFR fully
blanketed sphere.
Nuclear calculations. The values of the parameters investigated were
RP {(core) = 0.03, 0.09, 0.15,
Pp/P; = 0.10-0.50.
Since only a relative comparison was needed, all calculations were made
with a spherical core and complete 3-ft spherical blanket. The xenon poison
fraction was taken as 0.01, and the samarium steady-state value was com-
puted for each region in each case.
The fission-product poison level in the blanket cannot be determined
without first knowing the blanket processing cycle. As a first approach,
the breeding ratio for the hot clean conditions was used to determine the
cyele time from which the RP in the blanket was calculated as described
previously. The relative poison levels determined on this basis were as
follows:
Pg/P; RP (blanket)
10% 0.029
25% 0.048
50% 0.155
24-2] TWO-FLUID REACTOR DESIGN 875
750 T
T
700 — —
&
<
o
o
(=]
x 600 - —
=
z RP=0.15
[ye)
o™
z
RP=0.09
500 —
RP=0.03
450 I ] | i |
0 10 20 30 40 .50 60
Pg/P,
Fic. 24-6. Fuel concentration in core vs. Pg/P; for two-fluid LMFR fully blan-
keted sphere,
All eriticality calculations were performed using the specifications out-
lined 1 Article 24-2.2. Two-group diffusion theory was employed, and a
two-group. multiregion code was used for solving the diffusion equations.
A~ previously mentioned a 37-group spectral code was used to generate
the two-group coefficients. The critical concentration of fuel in the core
and blinket, breeding ratio, and neutron losses were determined for several
power =plits for each relative poison level in the core. The blanket power
fraction values of 10, 33.3, and 509 were used as reference values for com-
pari=oni, and the important nuclear parameters were determined from a set
of puranetric curves for these precise values. (Cases actually caleulated
corre=ponded very closely to the desired blanket power in most calecu-
lations-,
The nuclear parameters corresponding to these power splits are sum-
marized 11 Table 24-2. Figures 24-5 and 24-6 show the variation of
Noy Vg oin both the core and blanket as the blanket power fraction
changes. This atom ratio of U2 to bismuth in the blanket ranges from
233 x 1077 to 2420 X 1078 for Pp/P;=0.10 to 0.50. In the core the
Ny N ratio decreases approximately 209 over the same range. The
TABLE 24-2
Resurts oF NUCLEAR CALCULATIONS FOR VARIOUS Power SpLITS
Relative | Relative fi:’ oes A}:’ Crage
isc i N2a/Nri X 108 Nag/Npi X 108, ermal | thermal
Case | P/l POISOIL | POISON | pp 1y (ygq |t 23/ BI Mg ke | %8 Mgz, kg flux in flux in
in in (core) (blanket) core blanket
core blanket
system system
I(a)|0.10 0.03 | 0.029 |1.0256| 1.132 620 368.7 255 53.2 77X 1013 | 5.20 X 1013
(b) (.09 1.007 | 1.132 664 395 255 53.2 15 4.97
(e) 015 0.978 | 1.132 732 435 .4 255 53.2 425 467
II(a)[0.3333] 0.03 0.0475 [1.007 | 1.132 554 215.8 1150 317 .13 x 1043 | 2.61 x 1013
(b) 0.09 0.993 | 1.132 599 233.5 1190 328 .40 2.39
(e) 0.15 0.978 | 1.132 667 260 1230 334 71 2.23
IT1 (a)|0.50 0.03 | 0.155 [0.980 | 1.135 494 154 .8 2420 834 62 x 1013 | 1.28 x 1013
(b) 0.09 0.959 | 1.135 542 170 2670 920 72 1.01
(¢) 0.15 0945 | 1.135 590 185 2760 951 .19 0.97
9.8
XdNIS8 NDISHd HOILOVHAY TAAd TVLAW dIndrl
$Z 'dVHD]
24-2] TWO-FLUID REACTOR DESIGN 877
2.4
22 B
$2rcx10'"]5
20} -
Average Thermal Neutron Flux in Core,
o
!
RP== 0% |
RP=.15
12 . - :
¢ 0.1 02 03 0.4 0.5 6.0
Pg/Py
Fic. 24-7. Average thermal flux in core vs. Pg/P; for two-fluid LMFR based on
a fully blanketed sphere at 825 Mw.
values of the average thermal neutron flux in the core and blanket are
graphed in Figs. 24-7 and 24-8, and BR in Fig. 24-9.
Bismuth tnrentory. The primary system volumes for Pp/P;= 0.33 and
0.50 are based on a six-loop capsule design. Each loop contains a bismuth
inventory of 245 ft3. 1f 509 of the power is generated in the blanket,
three loops contain blanket slurry and three contain U-Bi core solution.
It one-third of the power originates in the blanket, two loops are devoted
to the blanket system and four to the core system. If only 10% of the total
power 1= venerated in the blanket, a three-loop design is assumed for the
core sv=rem, and two small loops of 125 ft3 each are used for the blanket.
The reactor holdup has been estimated from the reactor drawing in Fig.
24-1. Fuel inventory volumes are summarized in Table 24-3.
Using the value of $2.25/1b of bismuth, 129 annual fixed charges, and a
densitv of 613.5 Ib/ft? (9.83 g/ce), the annual bismuth inventory charges
are
(S yr) = 165.6 (Ves + Vis),
Wiiere
1'es = inventory volume of core system, ft3,
I'vs = Inventory volume of blanket system, ft3.
Foud toendory, Five days’ holdup of fuel from both blanket and core is
assumed ror the chemieal processing plant. Pa?33 is held up for 135 days to
allow for decav to U233, Approximately 3% of the Pa?33 remains after
135 days and ix discarded with the fission-product waste. This loss, while
878 LIQUID METAL FUEL REACTOR DESIGN STUDY [caAP. 24
f |
—
!
il
Average Thermal Neutron Flux in Blanket, 252 B X 10-14
10 —
0.8 —
RP=.03
06 —
RP=.09
RP=15
y L
0 0.1 0.2 0.3 0.4 0.5 0.6
Pp /Py
Fic. 24-8. Average thermal flux in blanket vs. Pg/P; for two-fluid LMFR
based on a fully blanketed sphere at 825 Mw.
1.03 T T
1.02 — ]
1.0 |
1.00 |- ]
0
£ 095 |- _
o
on
£
-
@
¢ 098 |- —]
om
0.97 = RP== 03]
0.96 |— ]
095 — —
RP=.09
RP==0.15
0.94 I | ] | l
0 A0 .20 .30 40 50 40
Fic. 24-9. Breeding ratio vs. Pp/P; for two-fluid LMFR fully blanketed sphere.
24-2] TWO-FLUID REACTOR DESIGN 879
TaBLE 24-3
INvENTORY VoLuMES IN Two-¥Fruip LMFR
Pp/P;=0.10 P,/P,=0.333 P/P.=0.50
Core svstem:
Reactor 275 ft3 275 ft3 275 ft3
External system 1640 980 735
Subtotal 1915 1255 1010
Blanket system:
Reactor ! 495 495 495
External svstem 250 490 735
Subtotal 745 985 1230
Total 2660 2240 2240
quite small, has been included with the fuel inventory charges, which may
be expressed as
(o (% vr =626 MG (1 + TO) + ME (1 + _T-S-) + 2 ME
b 1][233 Z13'
a Tg
(1 + 13;’,? 3) + 30 4 132,000
This equation assumes a 30-kg inventory of U233 feed material external
to the reactor. The economic assumptions used in this equation are 497
fuel fease charges and a U233 price of $15.65/g.
Foucl boirup. The annual cost of the net U232 fuel burned in an 825-Mw
reactor. a=suming an 809 plant factor, is
(3 ($/yr) = 3.96 X 10° (1 4+ a23)(1 — BR).
Thorinm amortization charges. Assuming a cost of $42,/kg for thorium
and an annual amortization rate of 159, based on a 20-yr life, the annual
amortization charges for the thorium are
Cy ($/yr) =6.3 Mys.
Thortiwm burnup. The thorium replacement costs due to burnup are cal-
culated according to the equation
05 ($/y1‘) = 10,620 (1 +0523) BR.
880 LIQUID METAL FUEL REACTOR DESIGN STUDY [cHAP. 24
3000 r I T I r T l r
B RP =15 7
| Blanket RS = 09 ]
—=——-Core RP = .03
1000 | T .
o [ - ——RP= .]SE
o = =
a [— —]
@ [ —_— ]
£ F e E
= = 4
® |— ]
~ — —
> L
o
o - 4
£
w — —
2
U
) _
& -
100 ]
5 -— 3
[— T ~—RP = 03—
501 | ] I ] I ] I L1 ]
Q.10 20 30 .40 .50 .60
Pg/Py
Fig. 24-10. Chemical processing cycles vs, blanket power, based on a blanketed
sphere with total reactor power of 825 Mw and the removal efficiencies of Z,, = 0.25,
Zy3=0.04, ZB = 0.10, ZEp = 1.00.
5x]06 T T T 1 T T 1 T T 1 T T T
1
B Total Annual Cost
-
‘“_: |
o
"; 1061 Capital Equipment ]
£ — -
g — i
3 — 7
° - . ]
s 6 — Operating Cost 3
T [— -
o —
£ _
c
L - i
I _
—
| Building Cost
10° ! [ bt P Lt bl !
1 3 6 10 30 60 100 200