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ORNL-1517.txt
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CENTRAL RESEA RCH 11
" DOCUMENT cpi L LIBRARY
S (T & - “PkLECTION
IVRURANER |
49555 4 e 2 )
S e 3 ORNL 1517 ey .44
3 .I 456 F EE Reactors-Research and Power @
ftas | ¢ ¥ AHEH ¥ neups
L' Q\\! | : N\
= NS | !w' % 5
:'3 ‘?{'}JI THE MODERATOR COOLIN s ' 8N
R ——
ke EL‘)P‘%‘ THE REFLECTOR-MODERATED REACTOR
6') R. W. Bussard
' W. S. Farmer o
H.
P
A, Fox
A, P. Fraas
By Av
br
CLASSIRICA TN cn“zi To: te o
CENTRAL RESEARCH LIBRARY
DOCUMENT COLLECTION
LIBRARY LOAN COPY
DO NOT TRANSFER TO ANOTHER PERSON
If you wish someone else to see this document,
send in name with document and the library will
arrange a loan,
OAK RIDGE NATIONAL LABORATORY
OPERATED BY
CARBIDE AND CARBON CHEMICALS COMPANY
A DIVISION OF UNION CARBIDE AND CARBON CORPORATION
(4 oy >
POST OFFICE BOX P
OAK RIDGE. TENNESSEE »
¥
ORNL 1517
%
£ ’ »
This documeht consists of 45 pages.
Copy4 of 165 copies. Series A.
Contract No. W-T405-eng-26
THE MODERATOR COOLING SYSTEM FOR THE
REFLECTOR-MODERATED REACTOR
R. W. Bussard A. H. Fox
W. S. Farmer A, P. Fraas
September 1953
DATE ISSUED
JAN 22 1954
OAK RIDGE NATIONAL LABORATORY
Operated by
CARBTIDE AND CARBON CHEMICALS COMPANY
A Division of Union Carbide and Carbon Corporation
Post Office Box P
‘r .
- LCRTRIGY AR
Osk Ridge, Tennessee
o ' 3 4455 D349555 4
- i1 - 3
ORNL 1517
Reactors-Research and Power
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THE MODERATOR COOLING SYSTEM FOR THE REFLECTOR-MODERATED REACTOR
R. W. Bussard A. H. Fox
W. S. Farmer A. P. Fraas
INTRODUCTION
Cooling the reflector region of the reflector-moderated circulating
fuel reactor presents an important set of problems. While reflector mate-
rials and coolants can be chosen independently of shielding considerations
for most types of reactor, this 1s not the case for an aircraft reactor
because the shield and i1ts weight are of such great importance. Not only
mist the reactor core be as small as possible but the reflector material
mist be chosen to give both a minimum fast neutron leakage from the reflec-
tor and a minimum production of hard secondary gammas in the reflector.
A number of reflector materials were considered on the basis of fast
neutron leakage per unit of thickness to get some notion of their influence
on shield design. (See Fig. 4.11 in ORNL-1515)1. This study showed that
beryllium was far superior to any of the other common reflector materials
such as beryllium oxide, carbon, or sodium deuteroxide, and 1t is somewhat
superior to Dp0. Although a fluid reflector might simplify the heat remov-
al problem, none of the fluid reflector materials that can be used at
temperatures of the order of 1000°F were comparable with beryllium for
neutron moderation and reflection. The reflector cooling problem was there-
fore studied using beryllium in order to evaluate the sources of heat
generation and the magnitude of their effects.
The design chosen for this study employed a fuel region in the form
of a thick-walled spherical shell of fuel with a beryllium reflector
surrounding 1t and a beryllium "island” filling the interior. The power
was taken as 200 megawatts and the core diameter as 18 in. giving a power
density 1in the fuel region of 5 kw/cm3 (see ORNL-15151, page 65). This
gave a source of radiation next to the reflector greater than that in any
existing reactor. (The MTR has a power density of 0.291 kw/cm3 in the
fuel region.)
SOURCES OF HEAT GENERATION
Heat wi1ll be generated in the reflector by the absorption of gamma
rays coming from the fuel and heat exchanger regions, and by the slowing
1. "ANP Quarterly Progress Report for Period Ending March 10, 1953,"
ORNL-1515.
down of fast fission neutrons. Approximately 12 Mev per fission was taken
as the total energy of the gamma rays generated in the fuel region. Of
this T.35 Mev was taken as representing fission fragment decay gammas with
an average photon energy of 1.5 Mev while 4.60 Mev was taken as coming
from prompt fission gammas with an average energy of(é°5 Mey.2 This choice
of gamma ray energy per fission has the effect of lumping all the fission
product decay gammas in the core. The distribution of decay gamma energy
between the core and heat exchanger regions depends upon the relative fuel
volumes of the regions, which varies with the detail design. As a first
approximetion all of the decay gamma energy was "lumped" in the core. For
such an assumption the estimate of the power density distribution in the
reflector will be somewhat higher and require more cooling close to the
fuel region than would be the case had the fission product decay gamma
energy been balanced between the core and heat exchanger regions. At the
same time "lumping" the decay gammas in the fuel region will yield an
underestimate of power density in the outer region of the reflector. It
is easy to correct for these effects later as will be shown (Appendix F).
Neutron capture results in the emission of a photon of approximately 9
Mev energy in the case of nickel and 6.8 Mev energy in the case of beryl-
lium.3 The kinetic energy of the neutrons amounts to approximately 5 Mev
per fission.
CALCULATION OF HEAT GENERATION
The ratio of peak to average power density appears to be fairly close
to unity i1n the three-region beryllium-reflected sodium-cooled reflector-
moderated reactor design. (See Table 4.1 - ORNL-1515)1. Therefore a
uniform power density and hence a uniform gamma source was assumed for
the fuel region in the first calculations. A later check using a non-
uniform power distribution from a multigroup calculation gave essentially
the same results.
In order to evaluate the self-absorption of gammas i1n the fuel region,
a typical fuel of sodium fluoride, potassium fluoride and UF) was
chosen for evaluating the absorption coefficient. (This does not mean
that the above fuel would necessarily be that specified finally for thas
reactor.) Gemma rays emtted in the fuel region cover a fairly wide
spectrum of energies with the mean value somewhere between 1 and 2.5 Mev.
Since heat generation was of principle concern, the mean energy was taken
2. "Estimested Heat Production in the NRU Reflector," CRT-50L.
3. E. P. Blizard, "Introduction to Shield Design," CF 51-10-70,
Part 1.
rI -‘ -6
‘
as 1 Mev i1n determining the absorption coefficient in the Inconel and
beryllium. This served to maximize the heat generation rate and gives a
limiting value. The absorption coefficient in the fuel region was also
evaluated at 1 Mev.
Since the elements in the reflector and fuel are principally of low
atomic number, Compton scattering 1s the principle mechanism for degrada-
tion of the gammas in the above energy range. The gamma rays were assumed
to be attenuated exponentially in calculating the heat generation. A
build-up factor was not employed since core diameter and reflector thick-
ness were small enough (of the order of one mean free path for 1 Mev
gammas) to make the need for a scattering correction questionable. It was
assumed that scattering would be straight ahead in direction and that
Compton collisions merely degrade the photon in energy. This method over-
estimates the gamma ray intensity for large distances.
An 18 in. diameter spherical fluoride fuel region surrounding a 9 in.
diameter central beryllium island and enclosed by a 12 in. thick beryllium
reflector were chosen as a typical geometry for calculation. The fuel
region was separated from the island and outer reflector by a shell of
3/16 in. thick Inconel. The reactor power output was taken as 200 mega-
watts 1n determining the total energy release. The neutron flux for
computing neutron capture gammas was taken from the spatial flux plot for
reactor calculation number 129 (see Table 4.1 ORNL-1515)1. The specific
heat generation rate was computed at points spaced about one inch apart
along the radius from the center of the 1sland to the outside of the
reflector.
The heat generation rate in the reflector arising from atfenuation
of the gamma rays emitted from the fuel region was computed by several
methods. In the first method (Appendix A) the attenuation was computed
taking into account numerical differences in the value of the absorption
coefficient of both fuel coolant, Inconel and beryllium. In Case A using
this method, the absorption coefficients employed were 0.09, 0.16, and
0.30 em-1, respectively, for the fuel, beryllium and Inconel regions. In
Case B values of 0.06 and 0.13 em-1 were used for the fuel and beryllium
regions, respectively, in order to evaluate the effect of the absorption
coefficient on the heat generation rate. The equation for exponential
attenuation using the above absorption coefficients was numerically
integrated to arrive at an answer for the heat generation rate at the
various space points. (Appendix A.) The results of this calculation
were checked by a method of graphical integration using Pappus' theorem.
(Appendix B.)
Another approach to the evaluation of the heat generation rate was
made by means of analytical solutions for exponential attenuation in terms
.
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of exponential integrals. A solution which would not involve graphical
or numerical integration could be obtained for two particular cases. By
assuming a uniform absorption coefficient throughout both the fuel and
the reflector regions, 1t is possible to solve the exponential integrals
directly. (Appendix C.) In the second case, the absorption coefficients
in the fuel region and reflector region were assumed to be different. An
approximaete solution can be obtained by solving the the problem in two
steps. The flux of gamma rays from the surface of the fuel region was
obtained using the uniform absorption coefficient solution method. The
attenuation through the Inconel was obtained by a slab source approxima-
tion. The resulting flux was then assumed to be spread over the surface
of the Inconel and the absorption in the reflector was determined for a
surface source. The results of this calculation are tabulated as Case C,
using the same absorption coefficients as in Case A.
The power density resulting from neutron moderation within the beryl-
lium of the island and reflector was obtained dire¢tly from multigroup
results by using the flux distribution §(r, M) or (¥nl)x C.F. (Correction
Factor)*. The energy loss for each lethargy group Nn/is the average energy
loss per collision times the number of collisions in that group at a given
radius or space point. The spatial distribution
_uli -u21
tn
7 W t —'}_ e -
10 1Z=1 _%_xC,F,, x f% ( e ) (1)
1s normalized to the total power lost by moderation (2 1/2% of reactor
power) by the use of the integration operator (1 (see ANP-58).
Gamma rays also result from parasitic capture of neutrons in struc-
tural materials and coolant. One particularly strong source of hard
gamma, rays is the Inconel shell separating the fuel annulus from the
outer reflector. These gammas are captured over an appreciable volume
rather than locally since the photon energy 1s high and the attenuation
length large. A minor amount of heating also results from the genera-
tion of gamma rays by neutron capture in the beryllium. The extent of
the captures in both beryllium and Inconel can be obtained directly from
the multigroup calculations or by using the integrated spatial neutron
flux distrabution weighted by the absorption probability. The latter
method was employed here. (Appendix D.)
REFLECTOR HEATING
The power density in the various regions of the reactor owing to
absorption of gamma rays from the core and reflector regions i1s tabulated
4. D. K. Holmes, "The Multigroup Method as Used by the ANP Physics
Group," ANP-58.
in Table I. The rate of heat generation is shown for Case A, Case B, and
Case C for the capture of gamms rays emitted in the fuel region. The last
column includes the heat generation rate caused by the capture of gamma
rays generated by parasitic neutron capture in beryllium plus those from
parasitic capture of neutrons in Inconel. Gamma rays will also result
from neutron captures in the coolant. These were not computed owing to
the uncertainty regarding the final coolant to be employed and the volume
fraction of the reflector that might be occupied by this coolant. Their
effect should be small, however. The power density resulting from the
slowing down of neutrons and gamma heating for Case A are plotted in Fig. 1.
The total integrated power in various regions from heating by gamma ray
absorption for Case A and Case B 1s shown in Table II.
Region
6
el
TABLE I
POWER DENSITY IN VARIOUS REGIONS
Island Beryllium
Island Inconel
Fuel
Reflector Inconel
Reflector Beryllium
Neutron
Radial Position Gamma. Heat Generation Capture
T Case A Case B Case C (n,d)
Cm. Watts/cm Watts/cm3
0 47.5 61.9 30 2.3
5.08 60 65 36 2.5
7.62 80 Th 6k 3.4
10.16 101 93 152 3.4
10.95 120 142 176 3.3
10.95 223 330 330 14,4
11.4 354 Lo7 koo 144
11.4 106 99 146
12.7 167 137
14 186 148
15.2 182 152
17.1 184 151
20.3 157 132
21.6 141 116
22.9 73 65 100
22.9 215 325 333 69.2
23.3 150 227 199 69.2
23.3 80 98 106 13.5
2k.1 23.7 27
25.4 37.7 4h .6 414.8 7.4
26.7 25.4 31.9
27.9 19.0 o4 L 17.4 5.0
30.5 10.3 1%.0
33.0 5.4 8.3 3.9 3.3
35.6 2.9 4.9
38.1 1.67 3.0 1.1 2.6
53.3 0.066 0.19
POWER DENSITY (watts /em®)
450
400
350
300
250
200
150
100
50
ISLAND
INCONEL SHELL
Na ANNULUS
INCONEL CAN
T ATING
TOTAL HE TOTAL HEATING
Y HEATING
NEUTRON
HEATING
Y HEATING
NEUTRON
HEATING
2 4 6 8
RADIAL DISTANCE FROM REACTOR CENTER LINE, » (1n)
Fig. 1. Radial Power Density from Neutron and Gamma Heating.
REFLECTOR
TOTAL HEATING
NEUTRON HEATING
y HEATING
10 12 14
16
18
DWG 187!!
20
i
«
AR
* -
£
kY
TOTAL INTEGRATED POWER IN VARIOUS REGIONS
Region
Island Beryllium
Island Inconel
Fuel
Reflector Inconel
Reflector Beryllium
— =
TABLE TI
Total Power Megawatts
Case A
0.46
0.24
6.71
0.57
3.14
Case B
0.51
0.29
5.58
0.85
3.44
The peak heat generation rate occurs in the Inconel shell separating
the 1sland beryllium from the fuel annulus. High heat generation rates
also occur in both the reflector and the i1sland immediately adjacent to
the fuel annulus. In cooling the Inconel core shells 1t 1s necessary to
take 1nto account not only the heat generation rate given in Table I, but
also the heat flowing through the Inconel from the fuel annulus when the
moderator region is designed to be operated at a lower temperature than
the fuel region. This can be computed readily by conventional methods.
COOLING SYSTEM
The heat generated in the Inconel and beryllium can be removed by
any one of several coolant passage arrangements. A liquid metal 1s the
most desirable coolant 1f the resulting heat is to be employed usefully
1n the engine air radiator circuit, since this gives the least sensitive
and highest heat transfer coefficient. Lead, bismuth or L1l might be
used 1n place of sodium because their effect on neutron moderation might
offer a certain nuclear advantage. The coolant chosen should not have
too high a neutron absorption cross-section (05.41_0.5b) and, what 1s
just as important, must be compatible with the materials of construction.
Lead, bismuth, non-uranium bearing fluorides, NaOH, sodium, and NaK were
all given serious consideration as coolants for the beryllium moderator.
Metallurgists consulted on the problem felt that lead or bismuth would be
likely to pose serious mass transfer difficulties. The relatively high
neutron absorption cross section of the potassium in the NaK made 1t quite
undesirable from the critical mass standpoint. Rubidium might be used 1in
place of potassium but because of little demand 1t 1is currently very
expensive. Thus sodium seemed to be the best choice for the moderator
coolant. Since corrosion and mass transfer might occur in a beryllium
and sodium system, 1t seemed desirable that the beryllium be clad in some
fashion. Work at Battelle5 indicates that beryllium can be chrome plated
electrolytically to give satisfactory resistance to sodium attack at
932°F. Chemical plating 1s also possible with beryllium. However, the
formation of brittle intermetallic compounds and the difficulty of elim-
inating pinholes with either chemical or electrical plating methods makes
the stability of any plating rather questionable under thermal cycling
and high temperature conditions. An alternate possibility 1s to can the
beryllium in thin-walled Inconel cans and to fill the small interstices
between the beryllium and the can with stagnant sodium to provide a
thermal bond. This arrangement appears to be the more promising of the
two, but both possibilities are being investigated. The reflector could
be constructed of two large hemispheres of beryllium if the canning
technique were used. Cooling passages could be rifle-drilled through
the beryllium and lined with thin-walled tubes, which could be welded
1nto headers at the ends. The Brush Beryllium Company has indicated that
5. J. G. Beach and C. L. Faust, "Electroplating on Beryllium," BMI-T732.
-]
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the fabrication of these large hemispherical shells would probably be no
more difficult than the fabrication of large flat slabs. Personnel of
the Y-12 beryllium shop state that 1t would not be difficult to rifle
drill holes 3/16 to 1/4 in. in diemeter as much as 40 1n. deep, with the
hole diameter held to within 0.001 in. and the hole center location held
to within 0.010 in. These holes could be drilled at a rate of 2 1n./m1n.
This estimate was based on the experience gained in machining the beryl-
lium of the MIR reactor and in drilling small diameter holes in the
beryllium reflector of the SIR. In addation to the holes in the beryl-
lium reflector, channels could be provided between the Inconel core shells
and the canned beryllium reflector in order to remove the heat generated
in this region.
An slternate construction for the reflector region involves the use
of a large number of wedge-shaped segments shaped much like the sections
of an orange. These sections could be made with shallow grooves in their
surfaces to form passages for cooling streams of sodium. This would be
a relatively expensive arrangement since a great deal of machine work
would be required because the beryllium can be hot-pressed to uniformly
high densities only in flat slabs or spherical shells.
A design study was made using the rifle-drilled hole arrangement to
investigate the detail problems of cooling the beryllium regions. The
beryllium was assumed to be canned in Inconel and cooled by sodium flow-
1ing through Inconel tubes in rifle-drilled holes. Stagnant sodium would
be allowed to fill the interstices between the beryllium and the can to
facilitate heat flow across that boundary. In order to achieve a well-
balanced design, & number of factors must be considered. The volume of
both the sodium and, especially, the Inconel must be minimized to keep
parasitic neutron absorptions within reasonable limits. It 1s also nec-
essary to operate the reflector regions at a relatively high temperature
to keep from penalizing the engine-radiator system. Large thermal stresses
are likely to result from the high rates of heat generation to be found in
these regions. Because beryllium becomes quite ductile at temperatures
sbove LOOPF cracking ought not be a problem. It was felt that thermal
stresses should be kept within reasonable limits to reduce distortion,
however, as this might become a problem after a number of thermal and/or
povwer cycles of the system. For this reason, the temperature variation
1n the beryllium between adjacent coolant passages was held to 50°F in
this first design. The pressure drop through the various coolant passages
was limited to 4O psi to keep pressure-induced stresses low. The maximum
beryllium-sodium interface temperature was held below 1200°F to minimize
the possibility of mass transfer in the beryllium-stagnant sodium-Inconel
systen.
smeliiiny
Several detail designs were investigated that favored first one and
then another of the various requirements, that 1s, minimum poison, minimum
variation in beryllium temperature, minimum beryllium-sodium interface
temperature variation, minimum sodium system pressure drop, etc. Fig. 2
shows the hole pattern in the beryllium for a promising arrangement. The
temperature distribution for this hole pattern i1s shown in Fig. 3.
ALTERNATE COOLING SYSTEMS
A careful examination of alternate cooling systems was made 1n an
effort to avoid the problems involved in cooling a solid beryllium island.
The sodium-cooled, solid beryllium outer reflector was assumed 1n every
casge.
The use of a semi-fluid beryllium powder mixture with a liquid metal
in the interstices was considered. A mln%mum porosity or liquid metal
volume fraction of 12% may be attainable. This would necessitate the use
of a liquid metal with a low neutron capture cross-section and good
"moderating" properties such as lead or bismuth. These are difficult to
contain, however, owing to corrosion and mass transfer. If a satisfactory
container material could be found, a semi-fluid moderator with a reasonably
small neutron age, [, would be attractive on the basis of ease of removal
for beryllium recovery and also as a safety measure.
Replacing the fuel annulus and i1sland by a graphite block containing
perhaps 40 unlined fuel passages about 1.5 in. in diameter has been proposed
as another possibility. The success of this system would depend largely on
whether the fuel could be kept from diffusing or penetrating into the
graphite as a result of permeation and/or cracking. If this were to occur,
severe overheating would result and self-destruction of the graphite would
take place. The destruction would be abetted by the large decrease in
thermal conductivity that accofipanles a temperature increase in graphite.
Actual testing of graphite in fused-fluoride, uranium-bearing salts under
conditions of thermal and mechanical shock will have to be made to evaluate
this problem. In addition, multigroup calculations will be necessary to
determine the critical mass and power dastribution. This latter item 1s
expected to be poor. Should Inconel tubes be required to protect the
graphite, a secondary cooling system would be required for cooling the
Inconel tube wall to 1500°F owing to the volumetric heat source effect.
If this were required the major advantage expected of graphite would be
lost.
A non-viscous fluid moderator for the i1sland with desirable heat trans-
fer properties would simplify the heat removal and the fabrication problems
6. M. Muskat, The Flow of Homogeneous Fluids Through Porous Media,
J. W. Edwards Company.
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3