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ORNL-3996.txt
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ORNL-3996.txt
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A_"_LORNL-3996
_';-IUC-SO Reactor Technology
" ‘BREEDER REACTORS
--‘-.:Pa'ul R -Kcst'en
E. S. Beths
Royic Roberrson
‘
'._?’;‘.‘},;.DESIGN ;STUDIE_S OF lOOO-Mw(e) MOLTEN sALT._’I-_ff_ff
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_;.‘.\‘\rv)|< AR
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Wil i loe )
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Pnnfed in USA. Pnce $5 00 Y Avu[lcbie from the Cleormghouse for Federcl
'5'7""7 s Sc:enhhc and Techpical informchon, Natienal Bureuu of Standards,®
' < VU.S. Depcrtrne,nf of Commer_ce__,_,_Spnngfn-cld,, V|rgmu_:r_ 22151 -
;nor the Commlsslcn, nor uny person nchng on behalf of fhe Comm:ssion.
or hus empleymeni vmh such confrector. SR
.Thls reporf was prepm‘ed as on account of Govefnment sponsored work Nelther fhe Umfed Sfctes,
' A“ Mokes any warrcnfy or represenioflon, sxpressed of |mphed “with reepecf to the cccuracy,
. completeness, ‘or - usefulness -of the informuhon ct:mh:unet:l m this report, or Ihat the vse of ~
any mformchon, cppcratus, rmefhod or process dnsclosed in Ihls report moy nof lnfrmge
privately owned nghfs, of oo e e : T
i "B, _':Assumes any Imb:lmes w:th respect to the ise of or for dqmages :esultmg from fhe use of
~ony mforrnchon, cppcrcfus, methed, ‘or procéss dlsclosed in this report. © T 0 -
i As used in the ‘abave, 'parson acting ‘on behalf of the Commlsslon mcludes any emp!oyee or 7
: '_;‘Vcontracfor of the Commlssmn, or employee of such confrucfor, to fl-ne extent thet - such employee
:ior confroctor of 'he Commlssion, or emplcyee of " such confracfor prepcres, dwsemmotes, or
' _:;provrdes access to, any Infermahon pursucnt to. I-ns employmenf or conircct w[!h tho Commasslon, S
Ay G v - (
CFSTI PRICES
/) o0
ne s 35.90; mugZ
ORNL-3996
Contract No. W-7405-eng-26
DESIGN STUDIES OF lOOO-Mw(e) MOLTEN-SALT BREEDER REACTORS
Paul R. Kasten
E. S. Bettis
Roy C. Robertson
Molten-Salt Reactor Program
R. B. Briggs, Director
W
RELEASED FOR ANNOUNCEMENT
| IN NUCLEAR SCIENCE ABSTRACTS
e b gt A
AUGUST 1966
OAK RIDGE NATIONAL LABORATORY
Oak Ridge, Tennessee
operated by
UNION CARBIDE CORPORATION
for the
U.S. ATOMIC ENERGY COMMISSION
«t
-
iii
SUMMARY
Design and evaluation studies have been made of thermal-energy
molten-salt breeder reactors (MSBR) in order to assess their economic and
nuclear performancehand to identify important design and development prob-
lems. The reference reactor design presented here is related to molten-
salt reactors in general.
The reference design is a two-region two-fluid system, with fuel salt
separated erm the_blanket salt by graphite tubes. The fuel salt consists
of uranium fluoride dissolved in a carrier salt of 1lithium and beryllium
fluorides, and the blanket salt contains thorium fluoride dissolved in a
similar carrier salt. The energy generated in the reactor fluid is trans-
ferred to a secondary coolant-salt cifcuit, which couples the reactor to a
supercritical steam cycle. On-site fuel-recycle processing is employed,
with fluoride-volatility and vacuum-distillation operations used for the
fuel fluid, and direct-protactinium-removal processing applied to the
blanket stream. The resulting power cost for the reference plant, termed
MSBR(Pa), is less than 2.7 mills/kwhr(e); the specific fissile-material
inventory is only 0.7 kg/Mw(e), the fuel doubling time is about 13 years,
and the fuel-cycle cost is 0.35 mill/kwhr(e). The associated power dou-
bling time based on continuous investment of bred fuel is less than 9
years.
Reference MSBR Plant Design
Flowsheet
Figure 1 gives the flowsheet of the lOOO-Mw(e) MSBR power plant.
Fuel flows through the reactor at a rate of about 44 OOO gpm (velocity of
about 15 fps); it enters the core at 1000°F and leaves at 1300°F. The
prlmary fuel C1rcuit hag four loops, and each loop has a pump and a pri-
mary heat exchanger. Each of these pumps has a capaC1ty of 'about 11,000
- gpm. The four blanket-ealt pumps and heat exchangers, although smaller,
are similar to corresponding components in thegfuei system. The blanket
salt enters the reactor vessel at 1150°F and leaves-at 1250°F. The
blanket-salt pumps have a capacity of about 2000 gpm.
REACTOR VESSEL
5.134 #
ORNL-DWG 66-7022
T 7
- 10.067 # 7.152¢ | 1518.5h-540p- 1000°
1550~ 1000*F - - |
1518.5h ! | i | 1424 h-3515p-1000° i
[ € l;— 1 ! i
r | 300p-1000°F | i GEN.
o ! 150 ft%sec L |20t Vs ! | : 52'(!;.2 Mwe
73ty 9.7 ¥ | BOILER | : | o o
= i2soer 1300°F REHEATERS< | | SUPERHEATERS 2s6In| 4 4
1150°F B50°F A J8s0°F Y 4 [ r
551.7° ' |
BLANKET SALT HEAT COOLANT SALT COOLANT SALT! ! GEN.
EXCH. AND PUMPS ' ; ;.
PUMPS PUMPS ' TURBINE [ TuriNg [] 3077 Mwe
FUEL SALT HEAT i ., | _ Gross
[uzsee EXGH. AND PUMPS g‘ @_“.f.'_”.a“ i ! r .
5. 5- | |
I T b T REHEAT STEAM oo
IIPE — i
LL'_[‘ T ! I | | PREHEATERS CONDENSER B FEEDWATER
| | ' = |' 3800p-7b0'F E 1307.8h SYSTEMS
| S | [te%2n 3500p-866°F <
o S| L __J i 3500p - 550.9°
J 1125°F hd v seash_ A Ao 234 | a0
f 0 570 p-GSO‘fi 3475p- 695°F
! eg—————— " j—
P — 766.4h
BOOSTER MIXING TEE
PUMPS
BLANKET SALT FUEL SALT COOLANT SALT PERFORMANCE
DRAIN TANKS DRAIN TANKS DRAIN TANKS NET OUTPUT 1000 Mwe
‘ LEGEND - GROSS GENERATION 1,034.9 Mwe
BF BOOSTER PUMPS 9.2 Mwe
FUEL == STATION AUXILIARIES 257 Mwe
BLANKET === wwe REACTOR HEAT INPUT 2225 Mwi
COOLANT —--— NET HEAT RATE 7,601 Blu/kwh
STEAM ———=—— NET "EFFICIENCY 449 %
o 10% 1b /hr
Pmmmmmn P8I0
Mo Bt /1b.
e .. Fraeze Valve
Fig. 1. Reference MSBR Flow Diagram
v
&4
o
oy
&
-
s -
Four 14,000-gpm pumps circulate the coolant, which consists of a mix-
ture of sodium fluoride and sodium fluoroborate. The coolant enters the
shell side of the primary heat exchanger at 850°F and leaves at 1112°F.
After leaving the primary heat exchanger, the coolant salt is further
heated to 1125°F on the shell side of the blanket heat exchangers. The
coolant then circulates through the shell side of 16 once-through super-
heaters (four superheaters per pump). In addition, four 2000-gpm pumps
circulate a portion of the coolant through eight reheaters.
The steam system flowsheet is essentially that of the new Bull Run
plant of the Tennessee Valley Authority system, with modifications to in-
crease the rating to 1000 Mw(e) and to preheat the working fluid to 700°F
prior to entering the heat exchanger-superheater unit. A supercritical
power-conversion system is used that is appropriate for molten-salt appli-
cation and takes advantage of the high-strength structural alloy employed.
Use of a supercritical fluid system results in an overall plant thermal
efficiency of about 45%.
Reactor Design
Figure 2 shows the plan and elevation views of the MSBR cell arrange-
ment. The reactor cell is surrounded by four shielded cells containing
the superheater and reheater units; these cells can be individually iso-
lated for maintenance. The fuel processing plant, located adjacent to
the reactor, is divided into high-level and low-level activity areas.
The elevation view in Fig. 2 indicates the position of equipment in the
various cells.
Figure 3 gives an elevation view of the reactor cell and shows the
- location of the reactor, pumps, and fuel and blanket heat exchangers.
The Hastelloy N reactor vessel has a side-wall thickness of about 1.25
in. and a head thickness of about 2.25 in.; it is designed to operate at
1200°F and up to 150 psi. The plenum chambers at the bottom of the ves-
sel commmnicate with the external heat exchangers by concentric inlet-
outlet piping. The inner pipe has slip joints to accommodate thermal
expansion. Bypass flow through these slip joints is about 1% of the
total flow. As indicated in Fig. 3, the heat exchangers are suspended
vi
from the top of the cell and are located below the reactor.
Each fuel
pump has a free fluid surface and a storage volume that permit rapid
drainage of fuel fluld from the core upon loss of flow. In addition,
the fuel salt can be drained to the dump tanks when the reactor is shut
down for an.extended time.
The entire reactor cell is kept at high tem-
perature, while cold "fingers" and thermal insulation surround structural
support members and all special equipment that must be kept at relatively
' REHEAT STEAM
ORNL-DWG 66=7111
1. e “ " '. o | i ’
H.P. STEAM -I‘l n " WASTE GAS N m n FEEDWATER
FEEDWATER 1| CELL o nn HP STEAM ,
fN0f. FUEL nn LP. STEAM 28
OOLANT SALT nil- )
¢ PUMPS ,’f-, « .{qn | HEAT EXCH [ rr{' fl :
et anl L o
Y AN DI et 4
2 = ; ‘ . i
B 0 X o 2 e
s v N 3 2 4
I = A 1
L2 — = ' 54 12 )
¢ : & 7 1 N
+ 8 REHEATERS
or .
AW L
1
é ‘7 ' ‘.” 2 ? v !
DEC(;I:’{)AQ_:%%‘Z@E ~. {j ) i 16 SUPERHEATERS
4 . ¢ BLANKET ,
; g - HEAT EXCH. 30
; ) B X CONTROL AREA—*
py S g e Tt s | T ¥
- 144 -
ORNL-DWG 66-7110
/ CONTROL ROD DRIVE
COOLANT SALT— FUEL CIRCULATING—, / BLANKET CIRCULATING
PUMPS —\ PUMP// ) ; / / PUMP
SUPERHEATERS—. _ ’
N
-
FUEL HEAT EXCH. Z REHEATERS
HEAT EXCH.
Fig. 2. Reactor and Coolant-Salt Cells — Plan and Elevation.
s
)
ORNL~DWG 66-7109
BLANKET PUMP
MOTCR
FUEL PUMP
MOTOR
CONTROL ROD
DRIVE
-
CONSTANT — £.07s
SUPPORT |~%:
HANGERS
w)
FUEL DUMP [ _
TANK WITH _. HERTTTT > Sl
COOLING =
COILS FOR
AFTER HEAT
REMOVAL
LANKET
et HEAT
' EXCH.
<
_____ e,
- -
. 2
AR :
2.
w 3 4
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' )
~
L TT—I0 FT. DIA
. CORE
'+ VESSEL
‘ a 4 .
l -‘ e .'.': o “ A "'"' b ‘l' ’ ’ o’ L d. .'” . L .' ':. : e R ’ 'l * L
. « " “REACTOR CELL HEATERS |, P I T e T, e
‘A_-. 'n_'.-.!\:l,l 04”\“ * P s * v _,s‘:-"'r
'Fig. 3. Reactor Cell — Elevation.
Ty
viii
low temperatures. The control rod drives are located above the core,
and the control rods are inserted into the central region of the core.
The reactor veséel, gbout 14 £t in diameter and about 19 ft high,
contains a 12.5-ft-high 10-ft-diam core assembly composed of reentry-
type graphite fuel elements. The graphite tubes are attached to the two
plenum chambers at the bottom of the reactor with graphite-to-metal
transition sleeves. Fuel from the entrance plenum flows up fuel passages
in the outer region of thé fuel tube and down through a single central
passage to the exit plenum. The fuel flows from the exit plenum to the
0
heat exchangers and then to the_pumprand back to the reactor. An 18-in.-
thick molten-salt blanket plus a 3~in.-thick graphite reflector surround .
the core. The blanket salt also permeates the interstices of the core
lattice, and thus fertile material flows through the core without mixing
with the fissile fuel salt. |
The MSBR requires structural integrity of the graphite fuel element.
In order to reduce the effect of radiation damage, the fuel tubes have
been made small to reduce the fast flux gradient across the graphite wall.
Also, the tubes are anchored only at one end to permit axial movement.
The core volume has been made large in order to reduce the flux level in
the core. In addition, the reactor is designed to permit replacement of
the entire graphite core by remote means if required. _
Figure 4 shows a cross section of a fuel element. Fuel fluid flows
upward through the small passages and downward through the large central .
passage. The outside diameter of a fuel tube is 3.5 in., and there are
534 of these tubes spaced on & 4.8-in. triangular pitch. The tube as- -
semblies are surrounded by hexagonal blocks of moderator graphite with
blanket salt filling the interstices. The nominal core composition is
75% graphite, 18% fuel salt, and 7% blanket salt by volume.
In determining the design parameters of the MSBR, two different
methods were considered for removal of bred fuel from the reactor. The
designation MSBR(Pa) represents a plant in which protactinium is removed
directly from the blanket stream, whereas the designation MSBR corre-
sponds to remcval of uranium per se from the blanket. With the exception
of the blanket-processing step, the MSBR(Pa) and the MSBR plants have (;J
essentially the same design. Development of an MSBR(Pa) plant is the '
')
)
Y
MODERATOR GRAPHITE)
FUEL PASSAGE (UP
ix
£ > ' ORNL~-DWG 66-7139
BLANKET PASSAGE
FUEL PASSAGE (DOWN)
35 OD. FUEL TUBE
MODERATOR HOLD
DOWN NUT GRAPHITE)
N
Al
o
§
3 REACTOR
| Wi S
- —SPACER
I 1 METAL TO GRAPHITE
- SLIP-JOINT
i-.‘___\.
—————METAL TO GRAPHITE
t - BRAZED JOINT
| | ——BRAZED JOINT
l —/
= .\ : r. Ny b=
= 2 \&E ~\. ——FUEL INLET
: i s PLENUM
= -
1 3 FUEL OUTLET
e re PLENUM
Fig. 4. MSBR Graphite Fuel Element.
present goal of the molten-salt reactor program. A summary of the
parameter values determined for the MSBR(Pa) and MSBR designs is given
in Table 1.
Fuel Processing
The primary objectives of fuel processing are to purify and recycle
fissile and carrier components and to minimize fissile inventory while
holding 1osses to a low value. The fluoride volatility—vacuum distilla-
tion process fulfills these objectives through simple operations. The
process for direct protactinium removal from the blanket also appears to
be a simple one. o |
The core fuel for both the MSBR and the MSBR(Pa) is processed by
fluoride volatility and vacuum distillation operations. For the MSER,
blanket processing is accomplished by fluoride volatility alone, and the
processing cycle time is short enough to maintain a very low concentraé
tion of fissile material. The effluent UFg is absorbed by fuel salt and
reduced to UF, by treatment with hydrogen to reconstitute a fuel-salt
mixture of the desired composition. For the MSBR(Pa), the blanket stream
is treated with molten bismuth containing dissolved thorium; the thorium
displaces the protactinium from solution (as well as uranium). The metal-
lie protactinium and uranium are deposited on a metal filter and hydro-
fluorinated or fluorinated for recyéle of bred fuel.
Molten-salt reactors are inherently suited to the design of process-
ing facilities integral with the reactor plant; these facilities require
only a small amount of cell space adjacent to the reactor cell. Because
all services and equipment available to the reactor are available to the
processing plant and shipping and storage charges are eliminated, inte-
gral processing facilities permit significant savings in capital and
dperating costs. Also, the processing plant inventory of fissile mate-
rial is very low.